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Site-Selective C–H Amination of Phenol-Containing Biomolecules
| dc.contributor.author | Girón-Elola, Carlota | |
| dc.contributor.author | Sasiain, Ibon | |
| dc.contributor.author | Sánchez-Fernández, Rosalía | |
| dc.contributor.author | Pazos, Elena | |
| dc.contributor.author | Correa, Arkaitz | |
| dc.date.accessioned | 2024-07-01T08:21:15Z | |
| dc.date.available | 2024-07-01T08:21:15Z | |
| dc.date.issued | 2023-06-07 | |
| dc.identifier.citation | Girón-Elola, C.; Sasiain, I.; Sánchez-Fernández, R.; Pazos, E.; Correa, A. Site-Selective C–H Amination of Phenol-Containing Biomolecules. Org. Lett. 2023, 25 (23), 4383–4387. https://doi.org/10.1021/acs.orglett.3c01560. | es_ES |
| dc.identifier.issn | 1523-7052 | |
| dc.identifier.issn | 1523-7060 | |
| dc.identifier.uri | http://hdl.handle.net/2183/37569 | |
| dc.description.abstract | [Abstract] A C–N bond-forming cross-dehydrogenative coupling of a collection of Tyr-containing peptides and estrogens with heteroarenes is described. This oxidative coupling is distinguished by its scalability, operational simplicity, and air tolerance and enables the appendance of phenothiazines and phenoxazines in phenol-like compounds. When incorporated into a Tb(III) metallopeptide, the Tyr-phenothiazine moiety acts as a sensitizer for the Tb(III) ion, providing a new tool for the design of luminescent probes. | es_ES |
| dc.description.sponsorship | We are grateful to Ministerio de Ciencia e Innovación (PID2021-122889NB-I00, CTQ2017-89166-R, MCIN/AEI/FEDER, UE), the Consellería de Cultura, Educación e Universidade, Xunta de Galicia (ED431C 2018/39, ED431C 2022/39, and 508/2020), and Basque Government (IT1741-22) for financial support. We thank for technical and human support provided by Central Service of Analysis-SGIker of UPV/EHU and European funding (ERDF and ESF). R.S.F. thanks the Consellería de Cultura, Educación e Universidade, Xunta de Galicia for her PhD fellowship (ED481A-2020/008). E.P. thanks the MCIN/AEI/10.13039/501100011033 and ESF Investing in your future for her RyC contract (RYC2019-027199-I) | es_ES |
| dc.description.sponsorship | Xunta de Galicia; ED431C 2018/39 | es_ES |
| dc.description.sponsorship | Xunta de Galicia; ED431C 2022/39 | es_ES |
| dc.description.sponsorship | Xunta de Galicia; 508/2020 | es_ES |
| dc.description.sponsorship | Gobierno Vasco; IT1741-22 | es_ES |
| dc.description.sponsorship | Xunta de Galicia; ED481A-2020/008 | es_ES |
| dc.language.iso | eng | es_ES |
| dc.publisher | American Chemical Society | es_ES |
| dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/PID2021-122889NB-I00/ES/NUEVAS APROXIMACIONES SINTETICAS EN LA FUNCIONALIZACION C-H DE PEPTIDOS | es_ES |
| dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/CTQ2017-89166-R/ES/HERRAMIENTAS PEPTIDICAS PARA APLICACIONES BIOLOGICAS: SENSORES INTELIGENTES PARA ESTUDIAR NITRACION DE PROTEINAS Y NANOMATERIALES CON FUNCIONALIDADES MODULABLES | es_ES |
| dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/RYC2019-027199-I/ES | es_ES |
| dc.relation.uri | https://doi.org/10.1021/acs.orglett.3c01560 | es_ES |
| dc.rights | Atribución 3.0 España | es_ES |
| dc.rights.uri | http://creativecommons.org/licenses/by/3.0/es/ | * |
| dc.title | Site-Selective C–H Amination of Phenol-Containing Biomolecules | es_ES |
| dc.type | info:eu-repo/semantics/article | es_ES |
| dc.rights.access | info:eu-repo/semantics/openAccess | es_ES |
| UDC.journalTitle | Organic Letters | es_ES |
| UDC.volume | 25 | es_ES |
| UDC.issue | 23 | es_ES |
| UDC.startPage | 4383 | es_ES |
| UDC.endPage | 4387 | es_ES |
| dc.identifier.doi | 10.1021/acs.orglett.3c01560 |
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