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Dynamic update of flow and transport parameters in reactive transport simulations of radioactive waste repositories
dc.contributor.author | Fernández Águila, Jesús | |
dc.contributor.author | Samper, Javier | |
dc.contributor.author | Mon, Alba | |
dc.contributor.author | Montenegro, Luis | |
dc.date.accessioned | 2024-01-30T17:34:18Z | |
dc.date.available | 2024-01-30T17:34:18Z | |
dc.date.issued | 2020 | |
dc.identifier.citation | Águila, J. F., Samper, J., Mon, A., Montenegro, L. (2020). Dynamic update of flow and transport parameters in reactive transport simulations of radioactive waste repositories. Applied Geochemistry, 117, 104585. https://doi.org/10.1016/j.apgeochem.2020.104585 | es_ES |
dc.identifier.uri | http://hdl.handle.net/2183/35249 | |
dc.description | Versión aceptada de https://doi.org/10.1016/j.apgeochem.2020.104585 | es_ES |
dc.description.abstract | [Abstract:] The changes in porosity caused by mineral dissolution/precipitation and the associated changes in flow, transport and chemical parameters of porous and fractured media are relevant for the geochemical time-evolution of natural and engineered underground systems. The realistic representation of natural systems requires modeling tools accounting for the changes in porosity. Here, we investigate the significance of the dynamic upgrade of the flow, transport and chemical parameters in reactive transport models with mineral dissolution/precipitation. The water flow, heat transfer and multicomponent reactive solute transport code, CORE2DV5, was extended to take into account the changes in porosity provoked by mineral dissolution/precipitation and their effect on flow, solute transport and chemical parameters. The improvements implemented in the code were verified against analytical solutions and the numerical solutions computed with other reactive transport codes with similar capabilities for isothermal mineral dissolution/precipitation test cases. Model results computed with CORE2DV5 agree with the analytical and numerical solutions for several isothermal test cases with porosity feedback. Model results show that failing to account for the porosity feedback leads to large errors. The porosity feedback effect (PFE) is especially relevant in long-term problems with mineral dissolution/precipitation leading to strong changes in porosity. The PFE is analysed with a non-isothermal geochemically-reactive transport model of the long-term (4·104 years) interactions of compacted bentonite with corrosion products and concrete in a high-level radioactive waste repository in clay. The model predicts pore clogging in the concrete and at the concrete-clay interface. The thickness of the zone affected by pore clogging computed with the PFE is smaller than that computed without the PFE. | es_ES |
dc.description.sponsorship | This work was funded by the CEBAMA Project of the European Atomic Energy Community's (Euratom) Horizon 2020 Programme (NFRP-2014/2015) under grant agreement # 662147, the Spanish Ministry of Economy and Competitiveness (Project CGL2016-78281), the FEDER funds, ENRESA (Spain), and the Xunta de Galicia (Galician Regional Government, project ED431C 2017/67). The first author enjoyed a Contract from the FPI Program of the Spanish Ministry of Economy and Competitiveness. We thank the comments and corrections of the three anonymous reviewers who contributed to the improvement of the paper. | es_ES |
dc.description.sponsorship | Xunta de Galicia; ED431C 2017/67 | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Elsevier | es_ES |
dc.relation | info:eu-repo/grantAgreement/EC/H2020/662147 | es_ES |
dc.relation | info:eu-repo/grantAgreement/MINECO/Plan Estatal de Investigación Científica y Técnica y de Innovación 2013-2016/CGL2016-78281-R/ES/MODELOS DE TRANSPORTE REACTIVO EN MEDIOS POROSOS CON ACTUALIZACION DINAMICA DE LOS PARAMETROS EN INTERFACES REACTIVAS | es_ES |
dc.relation.uri | https://doi.org/10.1016/j.apgeochem.2020.104585 | es_ES |
dc.rights | Atribución-NoComercial-SinDerivadas 3.0 España | es_ES |
dc.rights.uri | http://creativecommons.org/licenses/by-nc-nd/3.0/es/ | * |
dc.subject | Reactive transport model | es_ES |
dc.subject | CORE2DV5 | es_ES |
dc.subject | Porosity feedback effect | es_ES |
dc.subject | Pore clogging | es_ES |
dc.subject | Radioactive waste disposal | es_ES |
dc.subject | Non-isothermal | es_ES |
dc.title | Dynamic update of flow and transport parameters in reactive transport simulations of radioactive waste repositories | es_ES |
dc.type | info:eu-repo/semantics/article | es_ES |
dc.rights.access | info:eu-repo/semantics/openAccess | es_ES |
UDC.journalTitle | Applied Geochemistry | es_ES |
UDC.volume | 117 | es_ES |
UDC.startPage | 104585 | es_ES |
dc.identifier.doi | 10.1016/j.apgeochem.2020.104585 |
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