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dc.contributor.authorGutiérrez Fernández, Edgar
dc.contributor.authorScaccabarozzi, Alberto D.
dc.contributor.authorBasu, Aniruddha
dc.contributor.authorSolano, Eduardo
dc.contributor.authorAnthopoulos, Thomas D.
dc.contributor.authorMartín, Jaime
dc.date.accessioned2022-03-15T09:27:14Z
dc.date.available2022-03-15T09:27:14Z
dc.date.issued2022-01-05
dc.identifier.citationGutierrez-Fernandez, E., Scaccabarozzi, A. D., Basu, A., Solano, E., Anthopoulos, T. D., Martín, J., Y6 Organic Thin-Film Transistors with Electron Mobilities of 2.4 cm² V⁻¹ s⁻¹ via Microstructural Tuning. Adv. Sci. 2022, 9, 2104977. https://doi.org/10.1002/advs.202104977es_ES
dc.identifier.issn2198-3844
dc.identifier.urihttp://hdl.handle.net/2183/29996
dc.descriptionFinanciado para publicación en acceso aberto: Universidade da Coruña/CISUGes_ES
dc.description.abstract[Abstract] There is a growing demand to attain organic materials with high electron mobility, μe, as current reliable reported values are significantly lower than those exhibited by their hole mobility counterparts. Here, it is shown that a well-known nonfullerene-acceptor commonly used in organic solar cells, that is, BTP-4F (aka Y6), enables solution-processed organic thin-film transistors (OTFT) with a μe as high as 2.4 cm² V⁻¹ s⁻¹. This value is comparable to those of state-of-the-art n-type OTFTs, opening up a plethora of new possibilities for this class of materials in the field of organic electronics. Such efficient charge transport is linked to a readily achievable highly ordered crystalline phase, whose peculiar structural properties are thoroughly discussed. This work proves that structurally ordered nonfullerene acceptors can exhibit intrinsically high mobility and introduces a new approach in the quest of high μe organic materials, as well as new guidelines for future materials design.es_ES
dc.description.sponsorshipJ.M. thanks MICINN/FEDER for the Ramón y Cajal contract and the grant Ref. PGC2018-094620-A-I00). The Xunta de Galicia is also acknowledged for the grant Proyectos de Consolidación Ref. ED431F 2021/009. J.M and E.G.-F. acknowledge support through the European Union's Horizon 2020 research and innovation program, H2020-FETOPEN-01-2018-2020 (FET-Open Challenging Current Thinking), “LION-HEARTED′, grant agreement no. 828984. J.M would like to thank the financial support provided by the IONBIKE RISE project. This project has received funding from the European Union's Horizon 2020 research and innovation programme under the Marie Skłodowska-Curie grant agreement No 823989. The authors also thank the technical and human support provided by SGIker of UPV/EHU and the European funding (ERDF and ESF)es_ES
dc.description.sponsorshipXunta de Galicia; ED431F 2021/009es_ES
dc.language.isoenges_ES
dc.relationinfo:eu-repo/grantAgreement/EC/H2020/828984es_ES
dc.relationinfo:eu-repo/grantAgreement/EC/H2020/823989es_ES
dc.relationinfo:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PGC2018-094620-A-I00/ES/FASES VITREAS EN POLIMEROS SEMICONDUCTORES/
dc.relation.urihttps://doi.org/10.1002/advs.202104977es_ES
dc.rightsAttribution 4.0 International (CC BY 4.0)es_ES
dc.rights.urihttps://creativecommons.org/licenses/by/4.0/*
dc.subjectElectron mobilityes_ES
dc.subjectNonfullerene acceptorses_ES
dc.subjectOrganic thin-film transistorses_ES
dc.subjectPolymorphismes_ES
dc.titleY6 Organic Thin-Film Transistors with Electron Mobilities of 2.4 cm² V⁻¹ s⁻¹ via Microstructural Tuninges_ES
dc.typeinfo:eu-repo/semantics/articlees_ES
dc.rights.accessinfo:eu-repo/semantics/openAccesses_ES
UDC.journalTitleAdvanced Sciencees_ES
UDC.volume9es_ES
UDC.issue1es_ES
UDC.startPage1es_ES
UDC.endPage8es_ES
dc.identifier.doihttps://doi.org/10.1002/advs.202104977


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