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‘One-pot’ engineering of 0D carbon-based inorganic nanoarchitectonics for boosting multitasking catalytic activity
dc.contributor.author | Gómez Pérez, Inmaculada Jénnifer | |
dc.contributor.author | Hou, Heting | |
dc.contributor.author | Muñoz, Jose | |
dc.contributor.author | Romero, Nuria | |
dc.contributor.author | Sala, Xavier | |
dc.contributor.author | García-Antón, Jordi | |
dc.date.accessioned | 2024-08-14T07:56:34Z | |
dc.date.available | 2024-08-14T07:56:34Z | |
dc.date.issued | 2024 | |
dc.identifier.citation | Hou, H., Muñoz, J., Gómez, I. J., Romero, N., Sala, X., & García-Antón, J. (2024). ‘One-pot’ engineering of 0D carbon-based inorganic nanoarchitectonics for boosting multitasking catalytic activity. Materials Today Chemistry, 37. https://doi.org/10.1016/J.MTCHEM.2024.102021 | es_ES |
dc.identifier.uri | http://hdl.handle.net/2183/38584 | |
dc.description.abstract | [Abstract] Easy-to-make nanostructured materials that exhibit multitasking activity —while reducing the use of hazardous solvents throughout its architectural design— is a must to advance in the so-called Industry 4.0. Herein, a simple and eco-friendly ‘one-pot’ functionalization approach has been devised for synthesizing 0D carbon-based inorganic nanoarchitectonics made of carbon dots (CDs, as core carbon source) carrying two different inorganic building blocks, viz. quantum dots (CdSe@ZnS–QDs) and metal nanoparticles (Pt–NPs). As a proof-of-principle, the multi-catalytic activity of the resulting 0D Pt/QD/CD nanoarchitectonics by means of photoelectrocatalysis and sonocatalysis has been considered and compared with the pristine CD counterpart, demonstrating its suitability for boosting pivotal catalytic tasks like i) the photoelectrogeneration of hydrogen via hydrogen evolution reaction (HER), and ii) the sonodegradation of environmental pollutants (i.e., Rhodamine B) in water. Overall, this chemical approach is general and might be tailored for architecting alternative carbon-based heterostructures to enhance alternative multi-catalytic tasks. | es_ES |
dc.description.sponsorship | H. H. acknowledges the program of China Scholarships Council (No. 201908440337). X.S. thanks ICREA for the ICREA Academia Prize 2020. X.S. and J.G.-A. thank MINECO/FEDER for financial support (PID2019-104171RB-I00). J. M. is indebted to the Ramón y Cajal Program (RYC2021-033820-I Fellowship) funded by MCIN/AEI/10.13039/501100011033 and by the European Union “NextGenerationEU/PRTR”. I. J. G. acknowledges the Spanish Ministry of Universities for a Beatriz Galindo (BG22/000147) and Maria Zambrano funding (RSU.UDC.MZ09 [RSU.UDC.MZ11]) transferred by the European Union-Next GenerationEU. | es_ES |
dc.language.iso | eng | es_ES |
dc.publisher | Elsevier | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2017-2020/PID2019-103891RJ-I00/NANOMATERIALES CATALITICOS CONFECCIONADOS A MEDIDA PARA LA PRODUCCION DE COMBUSTIBLES SOLARES Y PRODUCTOS QUIMICOS DE VALOR AÑADIDO | es_ES |
dc.relation | info:eu-repo/grantAgreement/AEI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/RYC2021-033820-I/ES/MOL3DTRONICS: Molecularly Engineering 3D-Printed Programmable (Opto)Electronics: Biorecognition Systems, Logic Gates & Switching Memories | es_ES |
dc.relation | info:eu-repo/grantAgreement/MUNI/Plan Estatal de Investigación Científica y Técnica y de Innovación 2021-2023/BG22%2F00147/ES | es_ES |
dc.relation.uri | https://doi.org/10.1016/j.mtchem.2024.102021 | es_ES |
dc.rights | Attribution-NonCommercial 4.0 International CC BY-NC 4.0 | es_ES |
dc.rights.uri | http://creativecommons.org/licenses/by-nc/3.0/es/ | * |
dc.subject | Sonocatalysis | es_ES |
dc.subject | Photocatalysis | es_ES |
dc.subject | Carbon dots | es_ES |
dc.subject | Metal nanoparticles | es_ES |
dc.subject | Hydrogen evolution reaction | es_ES |
dc.title | ‘One-pot’ engineering of 0D carbon-based inorganic nanoarchitectonics for boosting multitasking catalytic activity | es_ES |
dc.type | info:eu-repo/semantics/article | es_ES |
dc.rights.access | info:eu-repo/semantics/openAccess | es_ES |
UDC.journalTitle | Materials Today Chemistry | es_ES |
UDC.volume | 37 | es_ES |
UDC.startPage | Artucle 102021 | es_ES |
dc.identifier.doi | 10.1016/j.mtchem.2024.102021 |